(a) An increase from $O^{2-}$ to $F^{-}$ and then decrease from $Na^+$ to $Al^{3+}$
(b) An decrease from $O^{2-}$ to $F^{-}$ and then increase from $Na^+$ to $Al^{3+}$
(c) An Significant increase $O^{2-}$ to $Al^{3+}$
(d) A significant decrease from $O^{2-} \; to \;Al^{3+} $